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1.
Int J Behav Nutr Phys Act ; 21(1): 36, 2024 Apr 02.
Artigo em Inglês | MEDLINE | ID: mdl-38566176

RESUMO

BACKGROUND: The Planetary Health Diet Index (PHDI) measures adherence to the dietary pattern presented by the EAT-Lancet Commission, which aligns health and sustainability targets. There is a need to understand how PHDI scores correlate with dietary greenhouse gas emissions (GHGE) and how this differs from the carbon footprints of scores on established dietary recommendations. The objectives of this study were to compare how the PHDI, Healthy Eating Index-2015 (HEI-2015) and Dietary Approaches to Stop Hypertension (DASH) relate to (a) dietary GHGE and (b) to examine the influence of PHDI food components on dietary GHGE. METHODS: We used life cycle assessment data from the Database of Food Recall Impacts on the Environment for Nutrition and Dietary Studies to calculate the mean dietary GHGE of 8,128 adult participants in the 2015-2016 and 2017-2018 cycles of the National Health and Nutrition Examination Survey (NHANES). Poisson regression was used to estimate the association of (a) quintiles of diet score and (b) standardized dietary index Z-scores with dietary GHGE for PHDI, HEI-2015, and DASH scores. In secondary analyses, we used Poisson regression to assess the influence of individual PHDI component scores on dietary GHGE. RESULTS: We found that higher dietary quality on all three indices was correlated with lower dietary GHGE. The magnitude of the dietary quality-dietary GHGE relationship was larger for PHDI [-0.4, 95% CI (-0.5, -0.3) kg CO2 equivalents per one standard deviation change] and for DASH [-0.5, (-0.4, -0.6) kg CO2-equivalents] than for HEI-2015 [-0.2, (-0.2, -0.3) kg CO2-equivalents]. When examining PHDI component scores, we found that diet-related GHGE were driven largely by red and processed meat intake. CONCLUSIONS: Improved dietary quality has the potential to lower the emissions impacts of US diets. Future efforts to promote healthy, sustainable diets could apply the recommendations of the established DASH guidelines as well as the new guidance provided by the PHDI to increase their environmental benefits.


Assuntos
Abordagens Dietéticas para Conter a Hipertensão , Gases de Efeito Estufa , Adulto , Humanos , Dieta Saudável , Gases de Efeito Estufa/análise , Inquéritos Nutricionais , Dióxido de Carbono/análise , Dieta
2.
J Environ Manage ; 357: 120736, 2024 Apr.
Artigo em Inglês | MEDLINE | ID: mdl-38574706

RESUMO

Onsite sanitation systems (OSS) are significant sources of greenhouse gases (GHG) including carbon dioxide (CO2), methane (CH4) and nitrous oxide (N2O). While a handful of studies have been conducted on GHG emissions from OSS, systematic evaluation of literature on this subject is limited. Our systematic review and meta-analysis provides state-of-the- art information on GHG emissions from OSS and identifies novel areas for investigation. The paper analyzes GHG emission rates from different OSS, the influence of various design, operational, and environmental factors on emission rates and proffers mitigation measures. Following the Preferred Reporting Items for Systematic reviews and Meta-analysis (PRISMA) guidelines, we identified 16 articles which quantified GHG emissions from OSS. Septic tanks emit substantial amounts of CO2 and CH4 ranging from 1.74 to 398.30 g CO2/cap/day and 0.06-110.13 g CH4/cap/day, respectively, but have low N2O emissions (0.01-0.06 g N2O/cap/day). CH4 emissions from pit latrines range from 0.77 to 20.30 g CH4/cap/day N2O emissions range from 0.76 to 1.20 gN2O/cap/day. We observed statistically significant correlations (p < 0.05) between temperature, biochemical oxygen demand, chemical oxygen demand, dissolved oxygen, storage period, and GHG emissions from OSS. However, no significant correlation (p > 0.05) was observed between soil volumetric water content and CO2 emissions. CH4 emissions (expressed as CO2 equivalents) from OSS estimated following Intergovernmental Panel for Climate Change (IPCC) guidelines were found to be seven times lower (90.99 g CO2e/cap/day) than in-situ field emission measurements (704.7 g CO2e/cap/day), implying that relying solely on IPCC guidelines may lead to underestimation of GHG emission from OSS. Our findings underscore the importance of considering local contexts and environmental factors when estimating GHG emissions from OSS. Plausible mitigation measures for GHG emissions from OSS include converting waste to biogas in anaerobic systems (e.g. biogas), applying biochar, and implementing mitigation policies that equally address inequalities in sanitation service access. Future research on GHG from OSS should focus on in-situ measurements of GHGs from pit latrines and other common OSS in developing countries, understanding the fate and transport of dissolved organics like CH4 in OSS effluents and impacts of microbial communities in OSS on GHG emissions. Addressing these gaps will enable more holistic and effective management of GHG emissions from OSS.


Assuntos
Gases de Efeito Estufa , Gases de Efeito Estufa/análise , Dióxido de Carbono/análise , Biocombustíveis/análise , Saneamento , Solo/química , Metano/análise , Óxido Nitroso/metabolismo , Efeito Estufa
3.
Sci Total Environ ; 926: 172133, 2024 May 20.
Artigo em Inglês | MEDLINE | ID: mdl-38569960

RESUMO

Evaluating the impact of global warming on rice production and greenhouse gas (GHG) emissions is critical for ensuring food security and mitigating the consequences of climate change. Nonetheless, the impacts of warming on crop production, GHG emissions, and microbial mechanisms in the single-cropping rice systems remain unclear. Here, a two-year field experiment was conducted to explore the effects of warming (increased by 2.7-3.0 °C on average) in the rice growing season on crop production and functional microorganisms associated with GHG emissions. Results showed that warming resulted in significant reduction (p < 0.01) in the aboveground biomass and grain yield as well as in grain weight, the number of spikelets per panicle, and the seed-setting rate. However, it caused a significant increase (p < 0.01) in the number of panicles by 15.6 % and 34.9 %, respectively. Furthermore, warming significantly increased (p < 0.01) seasonal methane (CH4) emissions but reduced nitrous oxide (N2O) emissions, particularly in 2022.The relative abundance of genes associated with CH4 metabolism and nitrogen metabolism was increased by 40.7 % and 32.7 %, respectively, in response to warming. Moreover, warming had a positive impact on the abundance of genes related to CH4 production and oxidation processes but did not affect the denitrification processes associated with N2O production. These results showed that warming decreased rice yield and biomass in the single cropping rice system but increased CH4 emissions and global warming potential. Taken together, to address the increasing food demand of a growing population and mitigate the impacts of global warming, it is imperative to duce GHG emissions and enhance crop yields.


Assuntos
Gases de Efeito Estufa , Oryza , Gases de Efeito Estufa/análise , Oryza/metabolismo , Agricultura/métodos , Aquecimento Global , Produção Agrícola , Óxido Nitroso/análise , Metano/análise , Solo , China
4.
PLoS One ; 19(4): e0297529, 2024.
Artigo em Inglês | MEDLINE | ID: mdl-38578792

RESUMO

Currently, the world faces an existential threat of climate change, and every government across the globe is trying to come up with strategies to tackle the severity of climate change in every way possible. To this end, the use of clean energy rather than fossil fuel energy sources is critical, as it can reduce greenhouse gas emissions and pave the way for carbon neutrality. This study examines the impact of the energy cleanability gap on four different climate vulnerabilities, such as ecosystem, food, health, and housing vulnerabilities, considering 47 European and non-European high-income countries. The study considers samples from 2002 to 2019. This study precedes the empirical analysis in the context of a quadratic relationship between the energy cleanability gap and climate vulnerability. The study uses system-generalized methods of the moment as the main technique, while panel quantile regression is a robustness analysis. Fixed effect and random effect models have also been incorporated. The study finds that the energy cleanability gap and all four climate vulnerabilities demonstrate a U-shaped relationship in both European and non-European countries, implying that when the energy cleanability gap increases, climate vulnerability decreases, but after reaching a certain threshold, it starts to increase. Development expenditure is found to be negatively affecting food and health vulnerabilities in European nations, while it increases food vulnerability and decreases health vulnerability in non-European nations. Regarding industrialization's impact on climate vulnerabilities, the study finds opposite effects for the European and non-European economies. On the other hand, for both groups, trade openness decreases climate vulnerabilities. Based on these results, the study recommends speeding up the energy transition process from fossil fuel energy resources towards clean energy resources to obtain carbon neutrality in both European and non-European groups.


Assuntos
Ecossistema , Gases de Efeito Estufa , Países Desenvolvidos , Gases de Efeito Estufa/análise , Desenvolvimento Econômico , Combustíveis Fósseis/análise , Carbono/análise , Dióxido de Carbono/análise , Energia Renovável
5.
Nat Commun ; 15(1): 3097, 2024 Apr 10.
Artigo em Inglês | MEDLINE | ID: mdl-38600111

RESUMO

The chemical transformations of methane (CH4) and carbon dioxide (CO2) greenhouse gases typically have high energy barriers. Here we present an approach of strategic coupling of CH4 oxidation and CO2 reduction in a switched microbial process governed by redox cycling of iron minerals under temperate conditions. The presence of iron minerals leads to an obvious enhancement of carbon fixation, with the minerals acting as the electron acceptor for CH4 oxidation and the electron donor for CO2 reduction, facilitated by changes in the mineral structure. The electron flow between the two functionally active microbial consortia is tracked through electrochemistry, and the energy metabolism in these consortia is predicted at the genetic level. This study offers a promising strategy for the removal of CH4 and CO2 in the natural environment and proposes an engineering technique for the utilization of major greenhouse gases.


Assuntos
Gases de Efeito Estufa , Gases de Efeito Estufa/análise , Dióxido de Carbono/análise , Oxirredução , Ferro , Metano/metabolismo , Minerais
6.
Sci Rep ; 14(1): 8706, 2024 04 15.
Artigo em Inglês | MEDLINE | ID: mdl-38622195

RESUMO

The sustainable management of leftover rice straw through biochar production to mitigate CH4 emissions and enhance rice yield remains uncertain and undefined. Therefore, we evaluated the effects of using biochar derived from rice straw left on fields after harvest on greenhouse gas emissions, global warming potential (GWP), and rice yield in the paddy field. The experiment included three treatments: chemical fertilizer (CF), rice straw (RS, 10 t ha-1) + CF, and rice straw-derived biochar (BC, 3 t ha-1 based on the amount of product remaining after pyrolysis) + CF. Compared with CF, BC + CF significantly reduced cumulative CH4 and CO2 emissions, net GWP, and greenhouse gas emission intensity by 42.9%, 37.4%, 39.5%, and 67.8%, respectively. In contrast, RS + CF significantly increased cumulative CH4 emissions and net GWP by 119.3% and 13.8%, respectively. The reduced CH4 emissions were mainly caused by the addition of BC + CF, which did not increase the levels of dissolved organic carbon and microbial biomass carbon, consequently resulting in reduced archaeal abundance, unlike those observed in RS + CF. The BC + CF also enhanced soil total organic carbon content and rice grain yield. This study indicated that using biochar derived from leftover rice straw mitigates greenhouse gas emissions and improves rice productivity in tropical paddy soil.


Assuntos
Carvão Vegetal , Gases de Efeito Estufa , Oryza , Solo/química , Aquecimento Global , Agricultura/métodos , Gases de Efeito Estufa/análise , Oryza/química , Metano/análise , Carbono , Óxido Nitroso/análise
7.
Sci Total Environ ; 927: 172270, 2024 Jun 01.
Artigo em Inglês | MEDLINE | ID: mdl-38583627

RESUMO

Recent studies show that greenhouse gas (GHG) emissions from urban landscape water are significant and cannot be overlooked, underscoring the need to develop effective strategies for mitigating GHG production from global freshwater systems. Calcium peroxide (CaO2) is commonly used as an eco-friendly reagent for controlling eutrophication in water bodies, but whether CaO2 can reduce GHG emissions remains unclear. This study investigated the effects of CaO2 dosage on the production of methane (CH4) and nitrous oxide (N2O) in urban landscape water under anoxic conditions during summer. The findings reveal that CaO2 addition not only improved the physicochemical and organoleptic properties of simulated urban landscape water but also reduced N2O production by inhibiting the activity of denitrifying bacteria across various dosages. Moreover, CaO2 exhibited selective effects on methanogens. Specifically, the abundance of acetoclastic methanogen Methanosaeta and methylotrophic methanogen Candidatus_Methanofastidiosum increased whereas the abundance of the hydrogenotrophic methanogen Methanoregula decreased at low, medium, and high dosages, leading to higher CH4 production at increased CaO2 dosage. A comprehensive multi-objective evaluation indicated that an optimal dosage of 60 g CaO2/m2 achieved 41.21 % and 84.40 % reductions in CH4 and N2O production, respectively, over a 50-day period compared to the control. This paper not only introduces a novel approach for controlling the production of GHGs, such as CH4 and N2O, from urban landscape water but also suggests a methodology for optimizing CaO2 dosage, providing valuable insights for its practical application.


Assuntos
Metano , Óxido Nitroso , Peróxidos , Qualidade da Água , Metano/análise , Óxido Nitroso/análise , Peróxidos/análise , Poluentes Químicos da Água/análise , Gases de Efeito Estufa/análise
8.
Sci Total Environ ; 927: 172296, 2024 Jun 01.
Artigo em Inglês | MEDLINE | ID: mdl-38588732

RESUMO

Constructed wetlands (CWs) are pivotal for wastewater treatment due to their high efficiency and numerous advantages. The impact of plant species and diversity on greenhouse gas (GHG) emissions from CWs requires a more comprehensive evaluation. Moreover, controversial perspectives persist about whether CWs function as carbon sinks or sources. In this study, horizontal subsurface flow (HSSF) CWs vegetated with Cyperus alternifolius, Typhae latifolia, Acorus calamus, and the mixture of these three species were constructed to evaluate pollutant removal efficiencies and GHG emissions, and estimate carbon budgets. Polyculture CWs can stably remove COD (86.79 %), NH4+-N (97.41 %), NO3--N (98.55 %), and TP (98.48 %). They also mitigated global warming potential (GWP) by suppressing N2O emissions compared with monoculture CWs. The highest abundance of the Pseudogulbenkiania genus, crucial for denitrification, was observed in polyculture CWs, indicating that denitrification dominated in nitrogen removal. While the highest nosZ copy numbers were observed in CWs vegetated with Cyperus alternifolius, suggesting its facilitation of denitrification-related microbes. Selecting Cyperus alternifolius to increase species diversity is proposed for simultaneously maintaining the water purification capacity and reducing GHG emissions. Carbon budget estimations revealed that all four types of HSSF CWs were carbon sinks after six months of operation, with carbon accumulation capacity of 4.90 ± 1.50 (Cyperus alternifolius), 3.31 ± 2.01 (Typhae latifola), 1.78 ± 1.30 (Acorus calamus), and 2.12 ± 0.88 (polyculture) kg C/m2/yr. This study implies that under these operation conditions, CWs function as carbon sinks rather than sources, aligning with carbon peak and neutrality objectives and presenting significant potential for carbon reduction efforts.


Assuntos
Gases de Efeito Estufa , Eliminação de Resíduos Líquidos , Áreas Alagadas , Gases de Efeito Estufa/análise , Eliminação de Resíduos Líquidos/métodos , Cyperus/metabolismo , Carbono/metabolismo , Águas Residuárias , Typhaceae/metabolismo , Acorus/metabolismo
9.
Lancet Planet Health ; 8 Suppl 1: S16, 2024 04.
Artigo em Inglês | MEDLINE | ID: mdl-38632911

RESUMO

BACKGROUND: There have been many modelled studies of potential health co-benefits from actions to reduce greenhouse gas emissions, but so far there have been no large-scale attempts to compare the magnitude of health and climate effects across sectors, countries, and study designs. METHODS: As part of the Pathfinder Initiative project an umbrella review of studies was done, and 26 previous reviews were identified with 57 primary studies included. Studies included in the review were required to have quantified changes in greenhouse gas emissions and health effects (or risk factors) from defined actions to reduce climate effects. Study data were extracted and harmonised by standardising impact measures per 100 000 of the national population (or urban population for city-level actions), averaging effects over a 1-year period and aggregating actions into their respective sectors by use of a predefined framework. FINDINGS: From 200 mitigation actions, the majority were in the agriculture, forestry, and land use sector (103 actions [52%]), followed by the transport sector (43 actions [22%]). The largest effects on greenhouse gas emissions were seen from actions in the energy sector, and these actions also had substantial health co-benefits in lower middle-income countries, although benefits were smaller in high-income settings. The greatest health benefits were seen from actions to change diets and introduce clean cookstoves. The major pathways to health were through reduced air pollution, healthier diets, and increased physical activity from switching to active travel modes. Effect sizes tended to be larger from national modelling studies and smaller from localised or implemented actions. INTERPRETATION: The potential co-benefits to health from actions to reduce climate change are large, but most evidence still comes from modelling studies and from high-income and middle-income countries. There are also major context-dependent differences in the magnitude of effects found, so actions need to be tailored to the local context and careful attention needs to be paid to potential trade-offs and spillover effects. FUNDING: The Wellcome Trust and the Oak Foundation.


Assuntos
Poluição do Ar , Gases de Efeito Estufa , Gases de Efeito Estufa/análise , Efeito Estufa , Poluição do Ar/análise , Agricultura
10.
Environ Monit Assess ; 196(5): 474, 2024 Apr 25.
Artigo em Inglês | MEDLINE | ID: mdl-38662125

RESUMO

Reducing emissions from deforestation and forest degradation (REDD) is a specific strategy for combating deforestation and forest degradation to alleviate the effects of climate change. In this study, the potential greenhouse gas (GHG) emission reduction resulting from the implementation of a REDD project is estimated. Changes in forest cover throughout the years 1985, 1990, 1995, 2000, 2010, 2015, and 2020 were analyzed using time-series Landsat imagery (TM, ETM + , and OLI) and a random forest algorithm. Multilayer perceptron neural networks were used to model the transition potential of the forest cover, which were then predicted via Markov chain analysis. The change detection analysis revealed two discernible patterns in forest cover dynamics. Between 1985 and 2000, a notable decrease in forest cover was seen, whereas from 2000 to 2020, it significantly increased. The results suggested that the absence of REDD implementation would result in the deforestation of approximately 199,569 hectares of forest cover between 2020 and 2050, leading to the release of 1,995,695 tCO2e of emissions into the atmosphere. However, with the implementation of REDD, these emissions would be reduced to 405,512 tCO2e, effectively preventing the release of 1,590,183 tCO2e of emissions into the upper atmosphere. This study demonstrates that the implementation of REDD projects can be an effective strategy for reducing GHG emissions and mitigating climate change in the Hyrcanian forests.


Assuntos
Mudança Climática , Conservação dos Recursos Naturais , Monitoramento Ambiental , Florestas , Gases de Efeito Estufa , Gases de Efeito Estufa/análise , Irã (Geográfico) , Conservação dos Recursos Naturais/métodos , Monitoramento Ambiental/métodos
11.
Sci Total Environ ; 924: 171484, 2024 May 10.
Artigo em Inglês | MEDLINE | ID: mdl-38462002

RESUMO

This study explores the greenhouse gas (GHG) fluxes of nitrous oxide (N2O), methane (CH4) and carbon dioxide (CO2) from a two-stage, cold-climate vertical-flow treatment wetland (TW) treating ski area wastewater at 3 °C average water temperature. The system is designed like a modified Ludzack-Ettinger process with the first stage a partially saturated, denitrifying TW followed by an unsaturated nitrifying TW and recycle of nitrified effluent. An intermittent wastewater dosing scheme was established for both stages, with alternating carbon-rich wastewater and nitrate-rich recycle to the first stage. The system has demonstrated effective chemical oxygen demand (COD) and total inorganic nitrogen (TIN) removal in high-strength wastewater over seven years of winter operation. Following two closed-loop, intensive GHG winter sampling campaigns at the TW, the magnitude of N2O flux was 2.2 times higher for denitrification than nitrification. CH4 and N2O emissions were strongly correlated with hydraulic loading, whereas CO2 was correlated with surface temperature. GHG fluxes from each stage were related to both microbial activity and off-gassing of dissolved species during wastewater dosing, thus the time of sampling relative to dosing strongly influenced observed fluxes. These results suggest that estimates of GHG fluxes from TWs may be biased if mass transfer and mechanisms of wastewater application are not considered. Emission factors for N2O and CH4 were 0.27 % as kg-N2O-N/kg-TINremoved and 0.04 % kg-CH4-C/kg-CODremoved, respectively. The system had observed seasonal emissions of 600.5 kg CO2 equivalent of GHGs estimated over 130-days of operation. These results indicate a need for wastewater treatment processes to mitigate GHGs.


Assuntos
Gases de Efeito Estufa , Purificação da Água , Gases de Efeito Estufa/análise , Áreas Alagadas , Dióxido de Carbono/análise , Efeito Estufa , Águas Residuárias , Monitoramento Ambiental , Nitrogênio , Metano/análise , Óxido Nitroso/análise
12.
Sci Total Environ ; 924: 171673, 2024 May 10.
Artigo em Inglês | MEDLINE | ID: mdl-38479519

RESUMO

Limited research has been conducted on ammonia (NH3) volatilization and greenhouse gases (GHGs) emissions in saline-alkali paddy fields, along with complex interaction involving various genes (16sRNA, amoA, narG, nirK, nosZ, and nifH). This study employed mesocosm-scale experiment to investigate NH3 volatilization and GHGs emissions, focusing on bacterial communities and genic abundance, in saline-alkali paddy fields with desulfurized gypsum (DG) and organic fertilizer (OF) amendments. Compared to the control (CK) treatment, DG and OF treatments reduced methane (CH4) and carbon dioxide (CO2) emissions by 78.05 % and 26.18 %, and 65.84 % and 11.62 %, respectively. However, these treatments increased NH3 volatilization by 26.26 % and 45.23 %, and nitrous oxide (N2O) emission by 41.00 % and 12.31 %. Notably, NH3 volatilization primarily stemmed from ammonia nitrogen (NH4+-N), rather than total nitrogen (TN) in soil and water. N2O was mainly produced from nitrate nitrogen (NO3--N) in soil and water, as well as NH4+-N in water. The increase in NH3 volatilization and N2O emission in DG and OF treatments, was attributed to the reduced competition among bacterial communities, rather than the increased bacterial activity and genic copies. These findings offer valuable insights for managing nutrient loss and gaseous emissions in saline-alkali paddy fields.


Assuntos
Gases de Efeito Estufa , Oryza , Solo , Dióxido de Carbono/análise , Amônia/análise , Álcalis , Gases de Efeito Estufa/análise , Nitrogênio/análise , Óxido Nitroso/análise , Fertilizantes/análise , Metano/análise , Água , Agricultura
13.
Environ Sci Technol ; 58(13): 5772-5783, 2024 Apr 02.
Artigo em Inglês | MEDLINE | ID: mdl-38502924

RESUMO

Under the "Double Carbon" target, the development of low-carbon agriculture requires a holistic comprehension of spatially and temporally explicit greenhouse gas (GHG) emissions associated with agricultural products. However, the lack of systematic evaluation at a fine scale presents considerable challenges in guiding localized strategies for mitigating GHG emissions from crop production. Here, we analyzed the county-level carbon footprint (CF) of China's rice production from 2007 to 2018 by coupling life cycle assessment and the DNDC model. Results revealed a significant annual increase of 74.3 kg CO2-eq ha-1 in the average farm-based CF (FCF), while it remained stable for the product-based CF (PCF). The CF exhibited considerable variations among counties, ranging from 2324 to 20,768 kg CO2-eq ha-1 for FCF and from 0.36 to 3.81 kg CO2-eq kg-1 for PCF in 2018. The spatiotemporal heterogeneities of FCF were predominantly influenced by field CH4 emissions, followed by diesel consumption and soil organic carbon sequestration. Scenario analysis elucidates that the national total GHG emissions from rice production could be significantly reduced through optimized irrigation (48.5%) and straw-based biogas production (18.0%). Moreover, integrating additional strategies (e.g., advanced crop management, optimized fertilization, and biodiesel application) could amplify the overall emission reduction to 76.7% while concurrently boosting the rice yield by 11.8%. Our county-level research provides valuable insights for the formulation of targeted GHG mitigation policies in rice production, thereby advancing the pursuit of carbon-neutral agricultural practices.


Assuntos
Gases de Efeito Estufa , Oryza , Solo , Carbono , Dióxido de Carbono/análise , Agricultura/métodos , Gases de Efeito Estufa/análise , Pegada de Carbono , China , Óxido Nitroso/análise
14.
Bioresour Technol ; 399: 130575, 2024 May.
Artigo em Inglês | MEDLINE | ID: mdl-38479629

RESUMO

Aerobic kitchen waste composting can contribute to greenhouse gas (GHGs) emissions and global warming. This study investigated the effects of biochar and zeolite on GHGs emissions during composting. The findings demonstrated that biochar could reduce N2O and CH4 cumulative releases by 47.7 %and 47.9 %, respectively, and zeolite could reduce the cumulative release of CO2 by 28.4 %. Meanwhile, the biochar and zeolite addition could reduce the abundance of potential core microorganisms associated with GHGs emissions. In addition, biochar and zeolite reduced N2O emissions by regulating the abundance of nitrogen conversion functional genes. Biochar and zeolite were shown to reduce the impact of bacterial communities on GHGs emissions. In summary, this study revealed that biochar and zeolite can effectively reduce GHG emissions during composting by altering the compost microenvironment and regulating microbial community structure. Such findings are valuable for facilitating high-quality resource recovery of organic solid waste.


Assuntos
Compostagem , Gases de Efeito Estufa , Zeolitas , Gases de Efeito Estufa/análise , Zeolitas/química , Solo/química , Metano/análise , Carvão Vegetal , Nitrogênio/análise , Óxido Nitroso/análise
15.
J Environ Manage ; 357: 120739, 2024 Apr.
Artigo em Inglês | MEDLINE | ID: mdl-38552522

RESUMO

Knowledge of freeze-thaw-induced carbon (C) and nitrogen (N) cycling and concomitant nitrous oxide (N2O) and carbon dioxide (CO2) emissions in perennial bioenergy crops is crucial to understanding the contribution of these crops in mitigating climate change through reduced greenhouse gas (GHG) emissions. In this study, a 49-day laboratory incubation experiment was conducted to compare the impact of freeze-thaw cycles on N2O and CO2 emissions in different perennial bioenergy crops [miscanthus (Miscanthus giganteus L.), switchgrass (Panicum virgatum L.), and willow (Salix miyabeana L.)] to a successional site and to understand the processes controlling the N2O and CO2 emissions in these crops. The results showed that freeze-thaw cycles caused a decline in dissolved organic C (DOC) and dissolved inorganic N (DIN) concentrations but enhanced the dissolved organic N (DON) and nitrate (NO3-). Although, freeze-thaw decreased water stable soil aggregates in all the bioenergy crops and successional site, this did not have any significant impact on N2O and CO2 emissions, suggesting that the N2O and CO2 emitted during the freeze-thaw cycles may have originated mostly from cellular materials released from lysis and death of microbial biomass rather than from soil aggregate disruption. Cumulative N2O emissions measured over the 49-day incubation period ranged from 148 mg N2O-N m-2 to 17 mg N2O-N m-2 and were highest in miscanthus followed by willow, switchgrass, and successional site. Cumulative CO2 on the other hand was highest in the successional site than any of the bioenergy crops and ranged from 25,262 mg CO2-C m-2 to 15,403 mg CO2-C m-2 after the 49 days. Higher N2O emissions in the miscanthus and willow than switchgrass and successional site were attributed to accelerated N losses as N2O. Results from our study indicate that managing perennial bioenergy crops on low productive agricultural lands to reduce freeze-thaw related GHG emissions and climate change mitigation is dependent on the crop species grown.


Assuntos
Gases de Efeito Estufa , Panicum , Gases de Efeito Estufa/análise , Dióxido de Carbono/análise , Agricultura/métodos , Solo , Óxido Nitroso/análise
16.
Biotechnol Adv ; 72: 108347, 2024.
Artigo em Inglês | MEDLINE | ID: mdl-38527656

RESUMO

Mitigating greenhouse gas emissions is a critical challenge for promoting global sustainability. The utilization of CO2 and CH4 as substrates for the production of valuable products offers a promising avenue for establishing an eco-friendly economy. Biocatalysis, a sustainable process utilizing enzymes to facilitate biochemical reactions, plays a significant role in upcycling greenhouse gases. This review provides a comprehensive overview of the enzymes and associated reactions involved in the biocatalytic conversion of CO2 and CH4. Furthermore, the challenges facing the field are discussed, paving the way for future research directions focused on developing robust enzymes and systems for the efficient fixation of CO2 and CH4.


Assuntos
Dióxido de Carbono , Gases de Efeito Estufa , Dióxido de Carbono/metabolismo , Biocatálise , Gases de Efeito Estufa/análise , Metano/metabolismo
17.
Sci Total Environ ; 926: 171962, 2024 May 20.
Artigo em Inglês | MEDLINE | ID: mdl-38537819

RESUMO

Estuaries are important components of the global carbon cycle; exchanging carbon between aquatic, atmospheric, and terrestrial environments, representing important loci for blue carbon storage and greenhouse gas emissions. However, how estuarine gradients affect sinking/suspended particles, and dissolved organic matter dynamic interactions remains unexplored. We fractionated suspended/sinking particles to assess and characterise carbon fate differences. We investigated bacterial colonisation (SYBR Green I) and exopolymer concentrations (TEP/CSP) with microscopy staining techniques. C/H/N and dry weight analysis identified particle composition differences. Meanwhile, nutrient and carbon analysis, and excitation and emission matrix evaluations with a subsequent parallel factor (PARAFAC) analysis characterised dissolved organic matter. The lack of clear salinity driven patterns in our study are presumably due to strong mixing forces and high particle heterogeneity along the estuary, with only density differences between suspended and sinking particles. Elbe estuary particles' organic portion is made up of marine-like (sinking) and terrestrial-like (suspended) signatures. Salinity did not have a significant role in microbial degradation and carbon composition, although brackish estuary portions were more biologically active. Indicative of increased degradation rates, leading to decreased greenhouse gas emissions, which are especially relevant for estuaries, with their disproportionate greenhouse gas emissions. Bacterial colonisation decreased seawards, indicative of decreased degradation, and shifts in microbial community composition and functions. Our findings span diverse strands of research, concerning steady carbon contributions from both marine and terrestrial sources, carbon aromaticity, humification index, and bioavailability. Their integration highlights the importance of the Elbe estuary as a model system, providing robust information for future policy decisions affecting dissolved and particulate matter dynamics within the Elbe Estuary.


Assuntos
Carbono , Gases de Efeito Estufa , Carbono/análise , Matéria Orgânica Dissolvida , Gases de Efeito Estufa/análise , Estuários , Material Particulado/análise , Rios
18.
Sci Total Environ ; 926: 172081, 2024 May 20.
Artigo em Inglês | MEDLINE | ID: mdl-38554961

RESUMO

Mature compost can promote the transformation of organic matter (OM) and reduce the emission of polluting gases during composting, which provides a viable approach to reduce the environmental impacts of biodegradable plastics (BPs). This study investigated the impact of mature compost on polybutylene adipate terephthalate (PBAT) degradation, greenhouse gas (GHG) emission, and microbial community structure during composting under two treatments with mature compost (MC) and without (CK). Under MC, visible plastic rupture was advanced from day 14 to day 10, and a more pronounced rupture was observed at the end of composting. Compared with CK, the degradation rate of PBAT in MC was increased by 4.44 % during 21 days of composting. Thermobifida, Ureibacillus, and Bacillus, as indicator species under MC treatment, played an important role in PBAT decomposition. Mature compost reduced the total global warming potential (GWP) by 25.91 % via inhibiting the activity of bacteria related to the production of CH4 and N2O. Functional Annotation of Prokaryotic Taxa (FAPROTAX) further revealed that mature compost addition increased relative abundance of bacteria related to multiple carbon (C) cycle functions such as methylotrophy, hydrocarbon degradation and cellulolysis, inhibited nitrite denitrification and denitrification, thus alleviating the emission of GHGs. Overall, mature compost, as an effective additive, exhibits great potential to simultaneously mitigate BP and GHG secondary pollution in co-composting of food waste and PBAT.


Assuntos
Plásticos Biodegradáveis , Compostagem , Gases de Efeito Estufa , Eliminação de Resíduos , Gases de Efeito Estufa/análise , 60659 , Alimentos , Solo/química , Metano/análise , Esterco
19.
Environ Sci Pollut Res Int ; 31(17): 25805-25822, 2024 Apr.
Artigo em Inglês | MEDLINE | ID: mdl-38491237

RESUMO

This paper examines the uncertainty of greenhouse gas (GHG) emissions during monorail construction. Firstly, a deterministic analysis is conducted. Subsequently, the obtained data are evaluated using the data quality indicator (DQI), and a Markov chain Monte Carlo (MCMC) simulation method is employed to assume different parameter distributions. The results of the deterministic calculation indicate that the calculated emissions per unit area of the station amount to 1.97 ton CO2e/m2, while the calculated emissions per unit section length reach 7.55 ton CO2e/m2. To simulate parameter distribution, we utilize a Beta distribution with good shape applicability. Furthermore, we establish scenarios involving system boundary reduction, low-emission factors, and reduced material and energy inputs in order to analyze scenario uncertainties. Regarding model uncertainty, this paper assumes that the material and energy quantity data conform to the normal, log-normal, uniform, and triangular distributions, respectively, subsequently analyzing the uncertainty distributions. This paper analyzes the GHG emission uncertainty evaluation of 16 monorail stations and sections during the construction period, which is divided into parameter, scenario, and model uncertainty. We provide a concrete framework for studying uncertainties related to GHG emissions at stations and sections during the monorail construction period. The scenario analysis results will help to make decisions about the choice of parameters, system boundaries, and other settings. It provides new guidance for emission reduction policies, such as reducing the use of steel-related products or using alternative environmentally friendly materials, considering emission reduction factors more comprehensively and setting emission reduction factors according to uniform distribution principle as far as possible.


Assuntos
Gases de Efeito Estufa , Gases de Efeito Estufa/análise , Incerteza , Efeito Estufa
20.
J Environ Manage ; 356: 120673, 2024 Apr.
Artigo em Inglês | MEDLINE | ID: mdl-38508003

RESUMO

Microplastics (MPs) accumulation in terrestrial ecosystems can affect greenhouse gases (GHGs) production by altering microbial and soil structure. Presently, research on the MPs effect on plants is not consistent, and underlying molecular mechanisms associated with GHGs are yet unknown. For the first time, we conducted a microcosm study to explore the impact of MPs addition (Raw vs. aged) and Trichoderma longibrachiatum and Bacillus subtilis inoculation (Sole vs. combination) on GHGs emission, soil community structure, physiochemical properties, and enzyme activities. Our results indicated that the addition of aged MPs considerably enhanced the GHGs emissions (N2O (+16%) and CO2 (+21%), respectively), C and N cycling gene expression, microbial biomass carbon, and soil physiochemical properties than raw MPs. However, the soil microbial community structure and enzyme activities were enhanced in raw MPs added treatments, irrespective of the MPs type added to soil. However, microbial inoculation significantly reduced GHGs emission by altering the expression of C and N cycling genes in both types of MPs added treatments. The soil microbial community structure, enzymes activities, physiochemical properties and microbial biomass carbon were enhanced in the presence of microbial inoculation in both type of MPs. Among sole and combined inoculation of Trichoderma and Bacillus subtilis, the co-applied Trichoderma and Bacillus subtilis considerably reduced the GHGs emission (N2O (-64%) and CO2 (-61%), respectively) by altering the expression of C and N cycling genes regardless of MPs type used. The combined inoculation also enhanced soil enzyme activities, microbial community structure, physiochemical properties and microbial biomass carbon in both types of MPs treatment. Our findings provide evidence that polyethylene MPs likely pose a high risk of GHGs emission while combined application of Trichoderma and Bacillus subtilis significantly reduced GHGs emission by altering C and N cycling gene expression, soil microbial community structure, and enzyme activities under MPs pollution in a terrestrial ecosystem.


Assuntos
Gases de Efeito Estufa , Microbiota , Gases de Efeito Estufa/análise , Solo/química , Microplásticos , Plásticos , Dióxido de Carbono/análise , Carbono , Bactérias , Óxido Nitroso/análise
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